"More allayed" typically means that someone is relieved or calmed down even further. Therefore, antonyms for this phrase could be words that mean the opposite, such as "agitated," "worried," "anxious," "fretful," or "restless." These words describe a state of heightened alertness or discomfort, the exact opposite of what someone feeling more allayed would be experiencing. Other antonyms could include words like "unsettled," "uneasy," "nervous," or "stressed," which all convey a sense of discomfort or anxiety, rather than relief or calmness. By using these antonyms, one could convey the opposite emotional state to that of feeling more allayed.