More contrarily can be synonymously expressed as "more oppositely", "more adversely", "more perversely", or "more differently". These terms indicate an intensified sense of opposition or contradiction, whether in a literal or figurative sense. They may be used to contrast contrasting ideas or behaviors, or simply to emphasize the unexpected or counterintuitive nature of a situation. While still conveying the essential meaning of "more contrarily", these synonyms allow for greater variety and nuance in language use, and can help to add complexity and texture to one's writing or speech.