The opposite of "more unagitated" can be described in several ways, such as restless, agitated, uneasy, anxious, or nervous. These antonyms suggest a state of discomfort, tension, or agitation, which contrasts with the calm, composed, and peaceful demeanor of someone who is more unagitated. The word "more" implies that the person or situation was already unagitated to some degree, and now there is a shift towards increased agitation or unrest. Depending on the context, the antonyms for "more unagitated" can convey different shades of meaning, such as a peaceful setting that is disrupted by noise or commotion, or a person who is normally calm but becomes tense in a stressful situation.