The word "more unaligned" implies a lack of alignment or cooperation between entities. Its antonym would be "aligned" or "coordinated," indicating a synchronized effort between two or more entities. Additionally, "harmonious," "complementary," and "compatible" are some synonyms that convey a sense of agreement and cooperation. These words imply that two or more entities are working together towards a common goal or objective, in a mutually beneficial way. Conversely, "divergent," "disjointed," and "conflicting" are related antonyms that suggest disagreement, disagreement, or disconnection. In both cases, the context and circumstances will determine which antonym is most appropriate.