The antonyms for the word "more rumpled" are "neat," "tidy," "orderly," "pressed," and "smooth." These words convey a sense of organization and cleanliness that is the opposite of a rumpled appearance. Neat and tidy imply a sense of order and arrangement, while orderly implies a systematic approach to arranging things. Pressed and smooth suggest a level of precision that is achieved through meticulous attention to detail. These antonyms can be useful when describing clothing, bedcovers, or even a person's appearance. By using these antonyms, you can create a sense of contrast and highlight the difference between a disheveled or chaotic state and an orderly and well-organized one.