The phrase "become less tolerable" means that something has started to bother or annoy us more than it used to. There are several synonyms for this expression, including "become unbearable," "become insupportable," "become intolerable," "become unendurable," and "become unpleasant."
When we use these words, we are indicating that the situation we are dealing with has reached a point where we can no longer handle it. We might say that the noise level in our office has become unbearable, or that the heat in our apartment has become insupportable. Whatever the situation, these synonyms help us convey the idea that we are at our wit's end and need a change.